Unveiling a critical point in glasses through high order non-linear measurements
Samuel Albert  1@  , Thomas Bauer  2@  , Marion Michl  2@  , Giulio Biroli  3@  , Jean-Philippe Bouchaud  4@  , Alois Loidl  2@  , Peter Lunkenheimer  2@  , Roland Tourbot  1@  , Cécile Wiertel-Gasquet  1@  , François Ladieu  1@  
1 : Service de physique de l'état condensé  (SPEC - CNRS / UMR 3680)  -  Website
CEA, CNRS : UMR3680
SPEC - CNRS / UMR 3680, CEA/Saclay, Orme des Merisiers, F-91191 GIF SUR YVETTE CEDEX -  France
2 : University of Augsburg, Germany
3 : IPhT CEA Saclay
4 : Capital Fund Management
Capital Fund Management

Although structural glasses are everyday materials playing an increasing role in modern technological applications [1], the glass transition in itself remains a conundrum. Over the two past decades several experimental breakthroughs have deepened our understanding of glasses. Among them, the developpement of third order non-linear response measurements [3,4,5,6,7] have been instrumental in putting forward new ways of measuring a significantly non-trivial thermodynamic response.
This talk will be devoted to showing how fifth order non-linear responses allows us to infer very strong experimental indications of the existence of a thermodynamic critical point in several archetypical glass formers [2]. Time permitting, various kinds of experimental nonlinear responses will be compared [3,4,5,6,7] with these results, aiming at giving a unified physical picture of the non-linear response in dielectric glass formers.

Acknowledgements

We thank C. Alba-Simionesco, A. Coniglio, P.-M. Déjardin, G. Tarjus, and M. Tarzia for interesting discussions. The work presented here was supported by ERC grant NPRGLASS, by the Labex RTRA grant Aricover, by the Institut des Systèmes Complexes ISC-PIF and by the Deutsche Forschungsgemeinschaft via Research Unit FOR1394.

References

[1] M. D. Ediger and P. Harrowell, J. Chem. Phys., 137, 080901 (2012).
[2] S. Albert, T. Bauer, M. Michl, G. Biroli, J.-P. Bouchaud, A. Loidl, P. Lunkenheimer, R. Tourbot, C. Wiertel-Gasquet, F. Ladieu, Science 352 (6291), 1308--1311 (2016).
[3] C. Crauste-Thibierge, C. Brun, F. Ladieu, D. L'Hôte, G. Biroli, J.-P. Bouchaud, Phys. Rev. Lett. 104, 165703 (2010).
[4] C. Brun, F. Ladieu, D. L'te, G. Biroli, J.-P. Bouchaud, Phys. Rev. Lett. 109, 175702 (2012).
[5] T. Bauer, P. Lunkenheimer, A. Loidl, Phys. Rev. Lett. 111, 225702 (2013)
[6] D. L'Hôte, R. Tourbot, F. Ladieu, P. Gadige, Phys. Rev. B 90, 104202 (2014).
[7] R. Casalini, D. Fragiadakis, C. M. Roland, J. Chem. Phys.142, 064504 (2015)


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